Auteur:
The Careful Programmer
Most of the games I like are puzzle-oriented, with a couple of action ones.
Let's start with the classical ones.
The Sudoku application from Mighty Mighty Good Games has the best interface of the ones I tried. I also actually thought I was pretty clever solving the expert level of the normal version until I bought the Expert Sudoku version and realized I sucked even at the easiest level. Their puzzles are hand crafted and often have a pleasing symmetrical quality.